In n = 1 RPP, the BA cations interlaced with each other due to interaction with apical I atom (shaded as red) of surface PbI6 octahedron, where by a larger in-plane octahedral tilt and a small out-of-plane tilt exist. In the case of n = 4 RPP, the BA molecules undertake a “head-to-head” configuration making sure that their NH3 groups ar

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